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The nearest access point to the highway is an elevator, south of Sunshine Tidings co-op.
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44 pistol may be found in an open safe in the upstairs rooms of the National Guard barracks. 44 pistol might be found inside a drawer in the Federal Surveillance Center K-21B in the south part of the map. 44 pistol may be found in Hardware Town on a table with a box and wine bottle in a room upstairs. Follow the pump pipe, it leads directly to the skeleton with the gun. Cross the bridge leaving Sanctuary then follow the shore left, past a dock until arriving at the water pump. The skeleton is leaning against a deactivated water pump not far from an unmarked small raider camp.
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A snubnosed version of this revolver can be found in the water filtration caps stash lying beside a skeleton close to the shore of the lake near Sanctuary, but before Concord is reached.
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